Meh, I have 3.23 gears and would not want anything more. It fits my engine perfectly with it's low revs and low to mid range torque. That being said, pick your gears to work with the engine you have and the intended driving. The 406 Camaro I put together for a friend a few years back had a 3.73/T-5 and 1st gear was practically unusable because it wound out too fast. The car was actually faster when we put in a 3.27 gear in it because it matched the car better. Plus, he didn't have to start in 2nd all the time. You have to consider the total effect of the compound gear ratio on the car and not just an initial feeling of acceleration. If the engine is high strung, it needs more gear to get off the line because it lacks the torque down low to get the car moving. With gearing, there can be too much of a good thing. If you make 400ft lbs at 1800 RPM, you really don't want more gear as it will just translate into tire smoke. If you only make 190 ft lbs like a stock 3.8 2bbl V6 or a high strung SBC (which can be even lower), you need more gear to get it moving because you need the extra multiplication. It also gets you to the power band faster and a high HP engine typically can handle the extra revs.
One of my current theoretical problems I am playing with on paper for fun is how to keep the fuel economy of an old Benz turbo diesel but improve it's dismal acceleration off the line. I came up with swapping from a stock 2.88 rear gear with 1:1 4th 4 speed auto and going with a 3.69 rear gear with a 0.8:1 5th in a 5 speed. It raises the final compound ratio to a 2.95 instead of a 2.88, but would let the car get off the line better to compensate for it's lackluster performance when it is out of boost (comes in at around 2500-3000). Compound first is now 14.74 vs 11.52 stock. In this case, shorter gears make more sense. I am also playing with a 2 stage turbo setup, propane injection and a water to air intercooler as other ways to improve initial acceleration--but I am getting off topic. Anyhow, just consider the engine and car it is in before choosing a gear.